Which preposition to use with granulate

in Occurrences 1%

The beating seems to do this, causing the dye to granulate in larger particles.

on Occurrences 1%

The lower half of what would otherwise be the oral opening of the cell is filled up by a thin plate of calcareous matter, granulated on the surface, and by which the actual opening is rendered more or less subtriangular, the mouth being placed just below the apex of the triangle.

Which preposition to use with  granulate